Search Results - "Jariwala, Sarthak"
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Tracking Photoexcited Carriers in Hybrid Perovskite Semiconductors: Trap-Dominated Spatial Heterogeneity and Diffusion
Published in ACS nano (28-11-2017)“…We use correlated confocal and wide-field fluorescence microscopy to probe the interplay between local variations in charge carrier recombination and charge…”
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The Role of Excitation Energy in Photobrightening and Photodegradation of Halide Perovskite Thin Films
Published in The journal of physical chemistry letters (19-04-2018)“…We study the impact of excitation energy on the photostability of methylammonium lead triiodide (CH3NH3PbI3 or MAPI) perovskite thin films. Light soaking leads…”
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3
Time-Resolved Electrical Scanning Probe Microscopy of Layered Perovskites Reveals Spatial Variations in Photoinduced Ionic and Electronic Carrier Motion
Published in ACS nano (26-03-2019)“…We study light-induced dynamics in thin films comprising Ruddlesden–Popper phases of the layered 2D perovskite (C4H9NH3)2PbI4. We probe ionic and electronic…”
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Polymer-modified halide perovskite films for efficient and stable planar heterojunction solar cells
Published in Science advances (01-08-2017)“…The solution processing of polycrystalline perovskite films introduces trap states that can adversely affect their optoelectronic properties. Motivated by the…”
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Reducing Surface Recombination Velocity of Methylammonium-Free Mixed-Cation Mixed-Halide Perovskites via Surface Passivation
Published in Chemistry of materials (13-07-2021)“…We control surface recombination in the mixed-cation, mixed-halide perovskite, FA0.83Cs0.17Pb(I0.85Br0.15)3, by passivating nonradiative defects with the…”
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Reducing Surface Recombination Velocities at the Electrical Contacts Will Improve Perovskite Photovoltaics
Published in ACS energy letters (11-01-2019)“…We explore the effects of nonradiative recombination at the extracting contacts on the achievable performance of halide perovskite photovoltaic cells. First,…”
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Interpreting Halide Perovskite Semiconductor Photoluminescence Kinetics
Published in ACS energy letters (14-06-2024)“…Drawing from both experimental data and simulation, we highlight best practices for fitting time-resolved photoluminescence (TRPL) decays of halide perovskite…”
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Dimethylammonium Addition to Halide Perovskite Precursor Increases Vertical and Lateral Heterogeneity
Published in ACS energy letters (14-01-2022)“…Adding a large A-site cation, such as dimethylammonium (DMA), to the perovskite growth solution has been shown to improve the performance and long-term…”
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9
Structure-Property Relationships in Organic-Inorganic Halide Perovskite Solar Cells
Published 01-01-2021“…Over the past 100 years, there has been a complete disregard for the environmental impact of unregulated burning of fossil fuels. This has led to an increase…”
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Dissertation -
10
Dimethylammonium Addition to Halide Perovskite Precursor Increases Vertical and Lateral Heterogeneity
Published in ACS energy letters (13-12-2021)“…Adding a large A-site cation, such as dimethylammonium (DMA), to the perovskite growth solution has been shown to improve the performance and long-term…”
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11
Dimethylammonium Addition to Halide Perovskite Precursor Increases Vertical and Lateral Heterogeneity
Published in ACS energy letters (13-12-2021)Get full text
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12
Controlling Spatial Crystallization Uniformity and Phase Orientation of Quasi‐2D Perovskite‐Based Light‐Emitting Diodes Using Lewis Bases
Published in Advanced materials interfaces (01-02-2020)“…Crystallographic orientation has a significant impact on the optoelectronic properties of films of quasi‐2D perovskite quantum wells. Here, oxygen‐bearing…”
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Quasi‐2D Perovskites: Controlling Spatial Crystallization Uniformity and Phase Orientation of Quasi‐2D Perovskite‐Based Light‐Emitting Diodes Using Lewis Bases (Adv. Mater. Interfaces 2/2020)
Published in Advanced materials interfaces (07-02-2020)“…The stability of intermediate complexes formed by the addition of Lewis bases is a key factor in modulating orientation of quasi‐2D perovskites as well as…”
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14
Dimethylammonium additives alter both vertical and lateral composition in halide perovskite semiconductors
Published 21-10-2021“…Adding a large A-site cation, such as dimethylammonium (DMA), to the perovskite growth solution has been shown to improve performance and long-term operational…”
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15
Approaching the limits of optoelectronic performance in mixed cation mixed halide perovskites by controlling surface recombination
Published 06-06-2020“…We demonstrate the critical role of surface recombination in mixed-cation, mixed-halide perovskite, FA0.83Cs0.17Pb(I0.85Br0.15)3. By passivating non-radiative…”
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16
Local Crystal Misorientation Influences Non-Radiative Recombination
Published 11-09-2019“…We use ultrasensitive electron backscatter diffraction (EBSD) to map the local crystal orientations, grains, and grain boundaries in CH3NH3PbI3 (MAPI)…”
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Journal Article