Search Results - "Jaramillo, Thomas F."

Molybdenum Phosphosulfide: An Active, Acid-Stable, Earth-Abundant Catalyst for the Hydrogen Evolution Reaction by Kibsgaard, Jakob, Jaramillo, Thomas F.

“…Introducing sulfur into the surface of molybdenum phosphide (MoP) produces a molybdenum phosphosulfide (MoP|S) catalyst with superb activity and stability for…”
Get full text

Engineering the surface structure of MoS2 to preferentially expose active edge sites for electrocatalysis by Kibsgaard, Jakob, Chen, Zhebo, Reinecke, Benjamin N., Jaramillo, Thomas F.

“…Controlling surface structure at the atomic scale is paramount to developing effective catalysts. For example, the edge sites of MoS 2 are highly catalytically…”
Get full text

Promoter Effects of Alkali Metal Cations on the Electrochemical Reduction of Carbon Dioxide by Resasco, Joaquin, Chen, Leanne D, Clark, Ezra, Tsai, Charlie, Hahn, Christopher, Jaramillo, Thomas F, Chan, Karen, Bell, Alexis T

“…The electrochemical reduction of CO2 is known to be influenced by the identity of the alkali metal cation in the electrolyte; however, a satisfactory…”
Get full text

Solar water splitting by photovoltaic-electrolysis with a solar-to-hydrogen efficiency over 30 by Jia, Jieyang, Seitz, Linsey C., Benck, Jesse D., Huo, Yijie, Chen, Yusi, Ng, Jia Wei Desmond, Bilir, Taner, Harris, James S., Jaramillo, Thomas F.

“…Hydrogen production via electrochemical water splitting is a promising approach for storing solar energy. For this technology to be economically competitive,…”
Get full text

Double layer charging driven carbon dioxide adsorption limits the rate of electrochemical carbon dioxide reduction on Gold by Ringe, Stefan, Morales-Guio, Carlos G., Chen, Leanne D., Fields, Meredith, Jaramillo, Thomas F., Hahn, Christopher, Chan, Karen

“…Electrochemical CO 2 reduction is a potential route to the sustainable production of valuable fuels and chemicals. Here, we perform CO 2 reduction experiments…”
Get full text

Electrocatalytic Conversion of Carbon Dioxide to Methane and Methanol on Transition Metal Surfaces by Kuhl, Kendra P, Hatsukade, Toru, Cave, Etosha R, Abram, David N, Kibsgaard, Jakob, Jaramillo, Thomas F

“…Fuels and industrial chemicals that are conventionally derived from fossil resources could potentially be produced in a renewable, sustainable manner by an…”
Get full text

Understanding activity trends in electrochemical water oxidation to form hydrogen peroxide by Shi, Xinjian, Siahrostami, Samira, Li, Guo-Ling, Zhang, Yirui, Chakthranont, Pongkarn, Studt, Felix, Jaramillo, Thomas F., Zheng, Xiaolin, Nørskov, Jens K.

“…Electrochemical production of hydrogen peroxide (H 2 O 2 ) from water oxidation could provide a very attractive route to locally produce a chemically valuable…”
Get full text

Electrochemical Ammonia SynthesisThe Selectivity Challenge by Singh, Aayush R, Rohr, Brian A, Schwalbe, Jay A, Cargnello, Matteo, Chan, Karen, Jaramillo, Thomas F, Chorkendorff, Ib, Nørskov, Jens K

Get full text

Core–shell MoO3–MoS2 Nanowires for Hydrogen Evolution: A Functional Design for Electrocatalytic Materials by Chen, Zhebo, Cummins, Dustin, Reinecke, Benjamin N, Clark, Ezra, Sunkara, Mahendra K, Jaramillo, Thomas F

“…We synthesize vertically oriented core–shell nanowires with substoichiometric MoO3 cores of ∼20–50 nm and conformal MoS2 shells of ∼2–5 nm. The core–shell…”
Get full text

Engineering Cu surfaces for the electrocatalytic conversion of CO2: Controlling selectivity toward oxygenates and hydrocarbons by Hahn, Christopher, Hatsukade, Toru, Kim, Youn-Geun, Vailionis, Arturas, Baricuatro, Jack H, Higgins, Drew C, Nitopi, Stephanie A, Soriaga, Manuel P, Jaramillo, Thomas F

“…In this study we control the surface structure of Cu thin-film catalysts to probe the relationship between active sites and catalytic activity for the…”
Get full text

Substrate selection for fundamental studies of electrocatalysts and photoelectrodes: inert potential windows in acidic, neutral, and basic electrolyte by Benck, Jesse D, Pinaud, Blaise A, Gorlin, Yelena, Jaramillo, Thomas F

“…The selection of an appropriate substrate is an important initial step for many studies of electrochemically active materials. In order to help researchers…”
Get full text

Designing Boron Nitride Islands in Carbon Materials for Efficient Electrochemical Synthesis of Hydrogen Peroxide by Chen, Shucheng, Chen, Zhihua, Siahrostami, Samira, Higgins, Drew, Nordlund, Dennis, Sokaras, Dimosthenis, Kim, Taeho Roy, Liu, Yunzhi, Yan, Xuzhou, Nilsson, Elisabeth, Sinclair, Robert, Nørskov, Jens K, Jaramillo, Thomas F, Bao, Zhenan

“…Heteroatom-doped carbons have drawn increasing research interest as catalysts for various electrochemical reactions due to their unique electronic and surface…”
Get full text

Understanding Selectivity for the Electrochemical Reduction of Carbon Dioxide to Formic Acid and Carbon Monoxide on Metal Electrodes by Feaster, Jeremy T, Shi, Chuan, Cave, Etosha R, Hatsukade, Toru, Abram, David N, Kuhl, Kendra P, Hahn, Christopher, Nørskov, Jens K, Jaramillo, Thomas F

“…Increases in energy demand and in chemical production, together with the rise in CO2 levels in the atmosphere, motivate the development of renewable energy…”
Get full text

Gas-Diffusion Electrodes for Carbon Dioxide Reduction: A New Paradigm by Higgins, Drew, Hahn, Christopher, Xiang, Chengxiang, Jaramillo, Thomas F, Weber, Adam Z

“…Significant advances have been made in recent years discovering new electrocatalysts and developing a fundamental understanding of electrochemical CO2…”
Get full text

Core–Shell Au@Metal-Oxide Nanoparticle Electrocatalysts for Enhanced Oxygen Evolution by Strickler, Alaina L, Escudero-Escribano, Marı́a, Jaramillo, Thomas F

“…Enhanced catalysis for electrochemical oxygen evolution is essential for the efficacy of many renewable energy technologies, including water electrolyzers and…”
Get full text

Standards and Protocols for Data Acquisition and Reporting for Studies of the Electrochemical Reduction of Carbon Dioxide by Clark, Ezra L, Resasco, Joaquin, Landers, Alan, Lin, John, Chung, Linh-Thao, Walton, Amber, Hahn, Christopher, Jaramillo, Thomas F, Bell, Alexis T

“…Objective evaluation of the performance of electrocatalysts for CO2 reduction has been complicated by a lack of standardized methods for measuring and…”
Get full text

Electrolyte Engineering for Efficient Electrochemical Nitrate Reduction to Ammonia on a Titanium Electrode by McEnaney, Joshua M, Blair, Sarah J, Nielander, Adam C, Schwalbe, Jay A, Koshy, David M, Cargnello, Matteo, Jaramillo, Thomas F

“…Nitrates from agricultural runoff and industrial waste streams are a notorious waste product and hazardous pollutant. Traditional electrochemical water…”
Get full text

Oxidation State and Surface Reconstruction of Cu under CO2 Reduction Conditions from In Situ X‑ray Characterization by Lee, Soo Hong, Lin, John C, Farmand, Maryam, Landers, Alan T, Feaster, Jeremy T, Avilés Acosta, Jaime E, Beeman, Jeffrey W, Ye, Yifan, Yano, Junko, Mehta, Apurva, Davis, Ryan C, Jaramillo, Thomas F, Hahn, Christopher, Drisdell, Walter S

“…The electrochemical CO2 reduction reaction (CO2RR) using Cu-based catalysts holds great potential for producing valuable multi-carbon products from renewable…”
Get full text

Machine-Learning Methods Enable Exhaustive Searches for Active Bimetallic Facets and Reveal Active Site Motifs for CO2 Reduction by Ulissi, Zachary W, Tang, Michael T, Xiao, Jianping, Liu, Xinyan, Torelli, Daniel A, Karamad, Mohammadreza, Cummins, Kyle, Hahn, Christopher, Lewis, Nathan S, Jaramillo, Thomas F, Chan, Karen, Nørskov, Jens K

“…Bimetallic catalysts are promising for the most difficult thermal and electrochemical reactions, but modeling the many diverse active sites on polycrystalline…”
Get full text

Understanding the Origin of Highly Selective CO2 Electroreduction to CO on Ni,N‐doped Carbon Catalysts by Koshy, David M., Chen, Shucheng, Lee, Dong Un, Stevens, Michaela Burke, Abdellah, Ahmed M., Dull, Samuel M., Chen, Gan, Nordlund, Dennis, Gallo, Alessandro, Hahn, Christopher, Higgins, Drew C., Bao, Zhenan, Jaramillo, Thomas F.

“…Ni,N‐doped carbon catalysts have shown promising catalytic performance for CO2 electroreduction (CO2R) to CO; this activity has often been attributed to the…”
Get full text