Optical properties of freestanding GaN nanomembranes using monochromated valence-EELS

[Display omitted] •The dielectric function of freestanding GaN nanomembranes is studied.•The dielectric function is described with the help of monochromated valence EELS.•Optical characteristics n, k, α and R are numerically deduced. In the present study, the dielectric function of freestanding GaN...

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Published in:Materials science & engineering. B, Solid-state materials for advanced technology Vol. 272; p. 115333
Main Authors: Benaissa, M., Sigle, W., Benabdallah, I., ElAfandy, R.T., Ng, T.K., van Aken, P.A.
Format: Journal Article
Language:English
Published: Lausanne Elsevier B.V 01-10-2021
Elsevier BV
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Summary:[Display omitted] •The dielectric function of freestanding GaN nanomembranes is studied.•The dielectric function is described with the help of monochromated valence EELS.•Optical characteristics n, k, α and R are numerically deduced. In the present study, the dielectric function of freestanding GaN nanomembranes was described using valence electron energy loss spectroscopy coupled to a monochromated electron probe in a Sub-Electron-volt Sub-Angstrom transmission electron Microscope. Such a technique has proven to be very efficient in handling nanometer-scale freestanding nanomembranes and provided local and direct measurements of optical characteristics. Indeed, core-state along with outer-shell electrons transitions were first measured in the configuration where the GaN c→-axis was normal to the transferred momentum q→. With the help of Kramers-Kroning analyses and density functional theory, critical points energies were extracted and assigned. Finally, optical data such as the real refractive index n, extinction coefficient k, absorption coefficient α and reflectivity R were numerically deduced from the real and imaginary parts of the dielectric function.
ISSN:0921-5107
1873-4944
DOI:10.1016/j.mseb.2021.115333