Search Results - "Duan, Lele"
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Selectively Etching Vanadium Oxide to Modulate Surface Vacancies of Unary Metal–Based Electrocatalysts for High‐Performance Water Oxidation
Published in Advanced energy materials (01-02-2020)“…Electrocatalytic water splitting for hydrogen generation is hindered by the sluggish kinetics of water oxidation, and highly efficient electrocatalysts for the…”
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Size‐Dependent Activity and Selectivity of Atomic‐Level Copper Nanoclusters during CO/CO2 Electroreduction
Published in Angewandte Chemie International Edition (04-01-2021)“…As a favorite descriptor, the size effect of Cu‐based catalysts has been regularly utilized for activity and selectivity regulation toward CO2/CO…”
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[2+1] Cycloadditions Modulate the Hydrophobicity of Ni‐N4 Single‐Atom Catalysts for Efficient CO2 Electroreduction
Published in Angewandte Chemie International Edition (15-07-2024)“…Microenvironment regulation of M‐N4 single‐atom catalysts (SACs) is a promising way to tune their catalytic properties toward the electrochemical CO2 reduction…”
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4
Novel Bi‐Doped Amorphous SnOx Nanoshells for Efficient Electrochemical CO2 Reduction into Formate at Low Overpotentials
Published in Advanced materials (Weinheim) (01-09-2020)“…Engineering novel Sn‐based bimetallic materials could provide intriguing catalytic properties to boost the electrochemical CO2 reduction. Herein, the first…”
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Synergizing Mo Single Atoms and Mo2C Nanoparticles on CNTs Synchronizes Selectivity and Activity of Electrocatalytic N2 Reduction to Ammonia
Published in Advanced materials (Weinheim) (01-08-2020)“…Previous research of molybdenum‐based electrocatalysts for nitrogen reduction reaction (NRR) has been largely considered on either isolated Mo single atoms…”
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Electronic Perturbation of Copper Single‐Atom CO2 Reduction Catalysts in a Molecular Way
Published in Angewandte Chemie International Edition (01-02-2023)“…Fine‐tuning electronic structures of single‐atom catalysts (SACs) plays a crucial role in harnessing their catalytic activities, yet challenges remain at a…”
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An amide-based second coordination sphere promotes the dimer pathway of Mn-catalyzed CO2-to-CO reduction at low overpotential
Published in Chemical science (Cambridge) (07-04-2021)“…The [fac-Mn(bpy)(CO)3Br] complex is capable of catalyzing the electrochemical reduction of CO2 to CO with high selectivity, moderate activity and large…”
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From Ru-bda to Ru-bds: a step forward to highly efficient molecular water oxidation electrocatalysts under acidic and neutral conditions
Published in Nature communications (14-01-2021)“…Significant advances during the past decades in the design and studies of Ru complexes with polypyridine ligands have led to the great development of molecular…”
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Second Sphere Effects Promote Formic Acid Dehydrogenation by a Single‐Atom Gold Catalyst Supported on Amino‐Substituted Graphdiyne
Published in Angewandte Chemie International Edition (06-03-2023)“…Regulating the second sphere of homogeneous molecular catalysts is a common and effective method to boost their catalytic activities, while the second sphere…”
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10
Visible Light-Driven Water Oxidation by a Molecular Ruthenium Catalyst in Homogeneous System
Published in Inorganic chemistry (04-01-2010)“…Discovery of an efficient catalyst bearing low overpotential toward water oxidation is a key step for light-driven water splitting into dioxygen and…”
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11
Dual Lewis Acid‐Base Sites Regulate Silver‐Copper Bimetallic Oxide Nanowires for Highly Selective Photoreduction of Carbon Dioxide to Methane
Published in Angewandte Chemie International Edition (25-09-2023)“…Highly selective photoreduction of CO2 to valuable hydrocarbons is of great importance to achieving a carbon‐neutral society. Precisely manipulating the…”
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Regulating Cu Oxidation State for Electrocatalytic CO2 Conversion into CO with Near‐Unity Selectivity via Oxygen Spillover
Published in Small (Weinheim an der Bergstrasse, Germany) (01-09-2024)“…Cu‐based catalysts are the most intensively studied in the field of electrocatalytic CO2 reduction reaction (CO2RR), demonstrating the capacity to yield…”
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13
Highly efficient and robust molecular ruthenium catalysts for water oxidation
Published in Proceedings of the National Academy of Sciences - PNAS (25-09-2012)“…Water oxidation catalysts are essential components of light-driven water splitting systems, which could convert water to H ₂ driven by solar radiation (H ₂O +…”
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14
Corrosion-Induced Cl-Doped Ultrathin Graphdiyne toward Electrocatalytic Nitrogen Reduction at Ambient Conditions
Published in ACS catalysis (06-12-2019)“…Electrochemical nitrogen fixation under ambient conditions is an attractive prospect to produce ammonia, yet the process still suffers from the sluggish…”
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Structural Modifications of Mononuclear Ruthenium Complexes: A Combined Experimental and Theoretical Study on the Kinetics of Ruthenium-Catalyzed Water Oxidation
Published in Angewandte Chemie (International ed.) (10-01-2011)“…Small change, big difference: A minor structural modification of water‐oxidation catalysts changes the kinetics of O2 evolution from second‐ to first‐order…”
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Single‐Site Heterogeneous Organometallic Ir Catalysts Embedded on Graphdiyne: Structural Manipulation Beyond the Carbon Support
Published in Small (Weinheim an der Bergstrasse, Germany) (01-11-2022)“…Accurate control over the coordination circumstances of single‐atom catalysts (SACs) is decisive to their intrinsic activity. Here, two single‐site…”
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17
Surface Functionalization of a γ‐Graphyne‐like Carbon Material via Click Chemistry
Published in Chemistry, an Asian journal (19-04-2021)“…Surface functionalization of carbon materials is of interest in many research fields, such as electrocatalysis, interfacial engineering, and supercapacitors…”
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Sacrificial W Facilitates Self‐Reconstruction with Abundant Active Sites for Water Oxidation
Published in Marine and petroleum geology (01-04-2022)“…Water oxidation is an important reaction for multiple renewable energy conversion and storage‐related devices and technologies. High‐performance and stable…”
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A nickel (II) PY5 complex as an electrocatalyst for water oxidation
Published in Journal of catalysis (01-03-2016)“…[Display omitted] A Ni-PY5 [PY5=2,6-bis(1,1-bis(2-pyridyl)ethyl)pyridine)] complex has been found to act as an electrocatalyst for oxidizing water to dioxygen…”
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Visible light-driven water oxidation catalyzed by mononuclear ruthenium complexes
Published in Journal of catalysis (01-10-2013)“…Visible light-driven water oxidation with high quantum efficiency of 17% has been achieved in homogeneous systems. [Display omitted] •Highly efficient…”
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