Evaporation temperature-tuned physical vapor deposition growth engineering of one-dimensional non-Fermi liquid tetrathiofulvalene tetracyanoquinodimethane thin films

We describe the growth of high quality tetrathiofulvalene tetracyanoquinodimethane (TTF-TCNQ) organic charge-transfer thin films which show a clear non-Fermi liquid behavior. Temperature dependent angle resolved photoemission spectroscopy and electronic structure calculations show that the growth of...

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Bibliographic Details
Published in:Applied physics letters Vol. 97; no. 11; pp. 111906 - 111906-3
Main Authors: Sarkar, I., Laux, M., Demokritova, J., Ruffing, A., Mathias, S., Wei, J., Solovyeva, V., Rudloff, M., Naghavi, S. S., Felser, C., Huth, M., Aeschlimann, M.
Format: Journal Article
Language:English
Published: American Institute of Physics 13-09-2010
Online Access:Get full text
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Summary:We describe the growth of high quality tetrathiofulvalene tetracyanoquinodimethane (TTF-TCNQ) organic charge-transfer thin films which show a clear non-Fermi liquid behavior. Temperature dependent angle resolved photoemission spectroscopy and electronic structure calculations show that the growth of TTF-TCNQ films is accompanied by the unfavorable presence of neutral TTF and TCNQ molecules. The quality of the films can be controlled by tuning the evaporation temperature of the precursor in physical vapor deposition method.
ISSN:0003-6951
1077-3118
DOI:10.1063/1.3489098