Full integration of highly stretchable inorganic transistors and circuits within molecular-tailored elastic substrates on a large scale

The emergence of high-form-factor electronics has led to a demand for high-density integration of inorganic thin-film devices and circuits with full stretchability. However, the intrinsic stiffness and brittleness of inorganic materials have impeded their utilization in free-form electronics. Here,...

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Published in:Nature communications Vol. 15; no. 1; p. 2814
Main Authors: Kang, Seung-Han, Jo, Jeong-Wan, Lee, Jong Min, Moon, Sanghee, Shin, Seung Bum, Choi, Su Bin, Byeon, Donghwan, Kim, Jaehyun, Kim, Myung-Gil, Kim, Yong-Hoon, Kim, Jong-Woong, Park, Sung Kyu
Format: Journal Article
Language:English
Published: London Nature Publishing Group UK 01-04-2024
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Summary:The emergence of high-form-factor electronics has led to a demand for high-density integration of inorganic thin-film devices and circuits with full stretchability. However, the intrinsic stiffness and brittleness of inorganic materials have impeded their utilization in free-form electronics. Here, we demonstrate highly integrated strain-insensitive stretchable metal-oxide transistors and circuitry (442 transistors/cm 2 ) via a photolithography-based bottom-up approach, where transistors with fluidic liquid metal interconnection are embedded in large-area molecular-tailored heterogeneous elastic substrates (5 × 5 cm 2 ). Amorphous indium-gallium-zinc-oxide transistor arrays (7 × 7), various logic gates, and ring-oscillator circuits exhibited strain-resilient properties with performance variation less than 20% when stretched up to 50% and 30% strain (10,000 cycles) for unit transistor and circuits, respectively. The transistors operate with an average mobility of 12.7 ( ± 1.7) cm 2 V −1 s −1 , on/off current ratio of > 10 7 , and the inverter, NAND, NOR circuits operate quite logically. Moreover, a ring oscillator comprising 14 cross-wired transistors validated the cascading of the multiple stages and device uniformity, indicating an oscillation frequency of ~70 kHz. Developing integrated stretchable metal-oxide transistors and circuits is challenging. Here, Kang et al. leveraged molecular-tailored elastic substrates for enhanced adhesion, thus achieving high performance and logical operation across various circuits under high strain.
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ISSN:2041-1723
2041-1723
DOI:10.1038/s41467-024-47184-w